Kuro Jujigun Soutou (Black Cross Fuehrer) He is the Black Cross' mysterious supreme leader, he was often referred to as the Machine Monster for his seeming invincible nature. He could not be easily killed by any conventional weapon. He had numerous supernatural powers and was incredibly intelligent. He kept his identity a secret even among his generals, by wearing a pointed white hooded robe but revealed his true form later on. In reality he was not even humanoid but rather a sentient alien machine construct who was part of the Black Cross Castle. He could also disguise himself as human, in either gender. He was finally defeated when the Goranger team combined their powers and launched their Cassiopeia Five Star attack.

Zolders Kuro Juujigun's faceless footsoldiers and loyaly brainwashed henchmen. Dressed from head to toe in black leather, these soldiers have been altered with enhanced strength and speed. They carry a variety of weapons including machine guns, bazookas and iron swords. Specialized divisions have also been created such as the Black Cross Army Camouflaged Ninja, who specialize in subversion and infiltration and the Africa Gundan, who are the elite soldiers who serve Golden Kamen Dai Shogun. There is also a squad of mystics who serve Kuro Juujigun Soutou and are adapt at the Black Arts. The Zolders could often be heard to be shouting Hoi when attacking their victims.

Sunring Mask He is the so-called 'Sun of Africa,' a ruthless tyrant who was renowned for his successive victories in Africa. He was called to Japan by Kuro Jujigun Soutou to help battle Goranger in Episode 15. Often used whatever means necessary to win. Often let his cowardly nature get in the way of his operations. He frequently battled one-on-one with Aka Ranger. He was efeated in his last duel with Aka Ranger through the Spear Whip and destroyed by the Goranger Storm in Episode 20. He could manipulate and generate intense fire at will, which he often focused through his staff.

General Iron Mask Temujin The second general, he was referred to as the Mongol Demon, he was recruited from Kuro Jujigun's Gobi Desert operations. He first appears in Episode 21. A cold and sadistic operative, he was a brilliant tactician and also formed his own army called the Steel Brigade (Tetsu Gundan). Vain and prideful, he often let his ego get in the way of his operations. He wielded a battle staff which ended in a sickle-like blade. He was virtually indestructible thanks to his steel armor, but ultimately, he was killed in Episode 42 when Aoranger controlled the Variblune remotely and the Goranger Storm balls that Temujin placed on his shoulders exploded in the Variblune cockpit, taking both Temujin and the Variblune with them.

General Firemountain Mask Magman He was Recruited from the volcanic Eldgja region in Iceland in Episode 42. Leader of the ruthless Funkan Gundan (Eruption Battalion). A cruel and calculating despot, he commanded his own mobile battle fortress dubbed Navarone, named after the Nazi Cannons off the Greek Aegean Islands in World War II. He had the ability to fire napalm missiles from the top of his volcano Mask. He was virtually impervious to Gorangers' weapons and was a master combatant. When the Goranger Machines were made to crash inside Navarone, it exploded from within taking him with it in Episode 52. His main attack was his Volcano Mask Rage Eruption.

Command in Chief Golden Mask He is the final general and Kuro Jujigun's top general. He is a supernatural entity that was mystically awoken in Episode 55 through Black Magic and Kuro Jujigun Soutou's powers. He is from Africa and resembles a pharaoh. He took command of Kuro Jujigun's elite African/Egyptian Troopers. Versed in sorcery and keenly interested in astrology. He could repel most of Gorangers' attacks and was near invincible. He was so fiercely loyal to Kuro Jujigun Soutou that he sacrificed his own life to reveal the location of Goranger headquarters, turning himself into a rainbow of gold dust. He also appeared in the 'Bomb Hurricane' movie.

Steel Sword Dragon He is a renegade Kuro Juujigun operative who was imprisoned by Kuro Juujigun Soutou for his recklessness and rebelliousness. Was later freed by Kuro Juujigun Soutou in exchange for his help in destroying Goranger. He was an incredibly strong fighter and was impervious to harm. He could easily repel the Goranger Hurricane attack, but the Gorangers managed to kill him with the Goranger Bomb Hurricane. He wielded the mighty Imperial Dragon Sword, which could cut and destroy almost any object. Appears in the movie 'Bomb Hurricane.'